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Advances in the development of a dissolution method for the attribution of iridium source materials

Title: Advances in the development of a dissolution method for the attribution of iridium source materials
Authors: Hodgson, APJ
Jarvis, KE
Grimes, RW
Marsden, OJ
Item Type: Journal Article
Abstract: To assist in nuclear forensic investigations, new techniques are required to evaluate radioactive materials that may be discovered outside of regulatory control. Using a recently developed pressure digestion method for iridium powder, assessments have been made of this techniques suitability for undertaking iridium target material evaluations. In addition to determining the reaction conditions necessary for total dissolution, these investigations have provided an insight into the elemental impurities that are present within unirradiated iridium targets that are used in QSA Global radiography sources, and established the speciation of the iridium solutions that are formed during this process.
Issue Date: 1-Feb-2017
Date of Acceptance: 1-Jan-2017
URI: http://hdl.handle.net/10044/1/69256
DOI: https://dx.doi.org/10.1007/s10967-016-5151-4
ISSN: 0236-5731
Publisher: Springer Verlag
Start Page: 1193
End Page: 1199
Journal / Book Title: Journal of Radioanalytical and Nuclear Chemistry
Volume: 311
Issue: 2
Copyright Statement: © The Author(s) 2017. This article is distributed under the terms of the Creative Commons Attribution 4.0 International License (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution, and reproduction in any medium, provided you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made.
Keywords: Science & Technology
Physical Sciences
Technology
Chemistry, Analytical
Chemistry, Inorganic & Nuclear
Nuclear Science & Technology
Chemistry
Iridium targets
Dissolution
Pressure vessels
Speciation
Nuclear forensics
PLATINUM-GROUP ELEMENTS
DIGESTION
0301 Analytical Chemistry
0302 Inorganic Chemistry
0306 Physical Chemistry (incl. Structural)
Inorganic & Nuclear Chemistry
Publication Status: Published
Conference Place: Budapest, HUNGARY
Online Publication Date: 2017-01-21
Appears in Collections:Materials
Faculty of Natural Sciences
Faculty of Engineering