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Estimating particulate exposure from modern Municipal Waste Incinerators (MWIs) in Great Britain.
File | Description | Size | Format | |
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Manuscript_clean.docx | Accepted version | 109 kB | Microsoft Word | View/Open |
Supporting Information_clean.docx | Accepted version | 3.14 MB | Microsoft Word | View/Open |
TOC Art.pdf | Accepted version | 108.13 kB | Adobe PDF | View/Open |
Title: | Estimating particulate exposure from modern Municipal Waste Incinerators (MWIs) in Great Britain. |
Authors: | Douglas, P Freni Sterrantino, A Leal Sanchez, M Ashworth, D Ghosh, R Fecht, D Font, A Blangiardo, M Gulliver, J Toledano, MB Elliott, P De Hoogh, C Fuller, GW Hansell, A |
Item Type: | Journal Article |
Abstract: | Municipal Waste Incineration (MWI) is regulated through the European Union Directive on Industrial Emissions (IED), but there is ongoing public concern regarding potential hazards to health. Using dispersion modeling, we estimated spatial variability in PM10 concentrations arising from MWIs at postcodes (average 12 households) within 10 km of MWIs in Great Britain (GB) in 2003–2010. We also investigated change points in PM10 emissions in relation to introduction of EU Waste Incineration Directive (EU-WID) (subsequently transposed into IED) and correlations of PM10 with SO2, NOx, heavy metals, polychlorinated dibenzo-p-dioxins/furan (PCDD/F), polycyclic aromatic hydrocarbon (PAH) and polychlorinated biphenyl (PCB) emissions. Yearly average modeled PM10 concentrations were 1.00 × 10–5 to 5.53 × 10–2 μg m–3, a small contribution to ambient background levels which were typically 6.59–2.68 × 101 μg m–3, 3–5 orders of magnitude higher. While low, concentration surfaces are likely to represent a spatial proxy of other relevant pollutants. There were statistically significant correlations between PM10 and heavy metal compounds (other heavy metals (r = 0.43, p = <0.001)), PAHs (r = 0.20, p = 0.050), and PCBs (r = 0.19, p = 0.022). No clear change points were detected following EU-WID implementation, possibly as incinerators were operating to EU-WID standards before the implementation date. Results will be used in an epidemiological analysis examining potential associations between MWIs and health outcomes. |
Issue Date: | 16-Jun-2017 |
Date of Acceptance: | 8-May-2017 |
URI: | http://hdl.handle.net/10044/1/48436 |
DOI: | https://dx.doi.org/10.1021/acs.est.6b06478 |
ISSN: | 0013-936X |
Publisher: | American Chemical Society |
Start Page: | 7511 |
End Page: | 7519 |
Journal / Book Title: | Environmental Science & Technology |
Volume: | 51 |
Issue: | 13 |
Copyright Statement: | © 2017 American Chemical Society |
Sponsor/Funder: | National Institute for Health Research Imperial College Healthcare NHS Trust- BRC Funding Medical Research Council (MRC) Medical Research Council (MRC) National Institute for Health Research Public Health England |
Funder's Grant Number: | NF-SI-0611-10136 RDC01 79560 MR/L01632X/1 MR/L01341X/1 RTJ6219303-1 6509268 |
Keywords: | Environmental Sciences MD Multidisciplinary |
Publication Status: | Published |
Appears in Collections: | School of Public Health |