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2D kaolin ultrafiltration membrane with ultrahigh flux for water purification

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Title: 2D kaolin ultrafiltration membrane with ultrahigh flux for water purification
Authors: Liu, T
Zhou, H
Graham, N
Yu, W
Sun, K
Item Type: Journal Article
Abstract: Membrane separation technology is an important option for the treatment of contaminated surface waters but the relatively high cost of materials and membrane fabrication represent a significant obstacle to the wider use of membrane processes. In this study, we describe the development and testing of a new kind of membrane made from two-dimensional (2D) kaolin nanosheets. The fabrication involved a layer-by-layer stacking of the nanosheets with a cationic polyacrylamide cross-linking agent, assembled on a cellulose acetate supporting layer. The kaolin membrane exhibited an ultrahigh flux (∼4000 L.m-2.h-1.bar-1) which was almost ten times greater than that of a commercial polyether sulfone (PES) ultrafiltration (UF) membrane. The membrane was tested using a range of influent water types, including samples of a lake water, river water and three natural organic matter solutions. The results showed that the kaolin membrane was stable and behaved as an UF membrane, in terms of its pore size distribution (peak distribution at 20-35 nm) and comparable treatment performance to the PES UF membrane. The kaolin membrane showed a substantially reduced rate of fouling, compared to PES membrane, despite a much greater flux, which was partly attributed to its highly hydrophilic nature. The advantages of lower cost, much higher flux and lower fouling propensity make the 2D-kaolin membrane a potentially important development in UF membrane technology for drinking water treatment, and possibly other applications.
Issue Date: 1-Jun-2019
Date of Acceptance: 25-Mar-2019
URI: http://hdl.handle.net/10044/1/70001
DOI: https://dx.doi.org/10.1016/j.watres.2019.03.050
ISSN: 0043-1354
Publisher: Elsevier
Start Page: 425
End Page: 433
Journal / Book Title: Water Research
Volume: 156
Copyright Statement: © 2019 Elsevier Ltd. All rights reserved. This manuscript is licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International Licence http://creativecommons.org/licenses/by-nc-nd/4.0/
Keywords: 2D material
Kaolin membrane
Ultrafiltration
Water treatment
2D material
Kaolin membrane
Ultrafiltration
Water treatment
Environmental Engineering
MD Multidisciplinary
Publication Status: Published
Conference Place: England
Embargo Date: 2020-03-26
Online Publication Date: 2019-03-26
Appears in Collections:Faculty of Engineering
Civil and Environmental Engineering



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