Self-potential during multiphase flow in complex porous media

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Title: Self-potential during multiphase flow in complex porous media
Authors: Zhang, Jiazuo
Item Type: Thesis or dissertation
Abstract: The rock pore space in many subsurface settings is saturated with water and one or more immiscible fluid phases; examples include non-aqueous-phase liquids (NAPLs) in contaminated aquifers, supercritical CO2 during sequestration in deep saline aquifers, the vadose zone, and hydrocarbon reservoirs. Self-potential (SP) methods have been proposed to monitor multiphase flow in such settings. However, to properly interpret and model these data requires an understanding of the saturation dependence of the streaming potential. This study presents a methodology to determine the saturation dependence of the streaming potential coupling coefficient and streaming current charge density in unsteady-state drainage and imbibition experiments and applies the method to published experimental data. Unsteady-state experiments do not yield representative values of coupling coefficient and streaming current density (or other transport properties such as relative permeability and electrical conductivity) at partial saturation because water saturation within the sample is not uniform. An interpretation method is required to determine the saturation dependence of coupling coefficient and streaming current density within a representative elementary volume with uniform saturation. The method makes no assumptions about the pore-space geometry. We also applied pore network models that can capture the distribution of fluids and electrical charge in real complex porous media to investigate and quantify streaming potential signals during multiphase flow at the pore level. The network modelling results were tested against the interpreted data and experimental data of Estaillades carbonate and St. Bees sandstone, which provided reliable pore-scale explanations of the experimental observations. The results presented here can be used to help interpret SP measurements obtained in partially-saturated subsurface settings.
Content Version: Open Access
Issue Date: Jan-2017
Date Awarded: Jun-2017
URI: http://hdl.handle.net/10044/1/48479
Supervisor: Jackson, Matthew
Vinogradov, Jan
Department: Earth Science & Engineering
Publisher: Imperial College London
Qualification Level: Doctoral
Qualification Name: Doctor of Philosophy (PhD)
Appears in Collections:Earth Science and Engineering PhD theses



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