Observing spin fractionalization in the Kitaev spin liquid via temperature evolution of indirect resonant inelastic x-ray scattering

Abstract

Motivated by the ongoing effort to search for high-resolution signatures of quantum spin liquids, we investigate the temperature dependence of the indirect resonant inelastic x-ray scattering (RIXS) response for the Kitaev honeycomb model. We find that, as a result of spin fractionalization, the RIXS response changes qualitatively at two well-separated temperature scales, T L and T H , which correspond to the characteristic energies of the two kinds of fractionalized excitations, Z 2 gauge fluxes and Majorana fermions, respectively. While thermally excited Z 2 gauge fluxes at temperature T L lead to a general broadening and softening of the response, the thermal proliferation of Majorana fermions at temperature T H ∼ 10 T L results in a significant shift of the spectral weight, both in terms of energy and momentum. Due to its exclusively indirect nature, the RIXS process we consider gives rise to a universal magnetic response and, from an experimental perspective, it directly corresponds to the K -edge of Ru 3 + in the Kitaev candidate material α − RuCl 3 .