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1D slipped stacking microribbon-like crystals based on 6,13-dicyanopentacene for ambipolar charge transport
File | Description | Size | Format | |
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Accepted manuscript.pdf | Accepted version | 1.07 MB | Adobe PDF | View/Open |
Title: | 1D slipped stacking microribbon-like crystals based on 6,13-dicyanopentacene for ambipolar charge transport |
Authors: | Wang, Z Hu, Y Xie, Y Qie, F Guo, J Zhang, L Shi, C Glöcklhofer, F Zhen, Y |
Item Type: | Journal Article |
Abstract: | Featuring small charge transport scattering, mesoscale size, and easy fabrication, one-dimensional self-assembled micro/nanomaterials (1D-MNMs) based on organic π-conjugated systems can be facilely incorporated into integrated microcircuits. Although tremendous progress has been made in 1D-MNMs based on p- or n-channel organic semiconductors, examples of lD-MNMs based on ambipolar organic semiconductors are scarce. Herein, we achieved a novel 1D-MNM based on 6,13-dicyanopentacene (DCP) with a 1D slipped stacking motif using the physical vapor transport method. The DCP-based 1D-MNM showed outstanding, well-balanced ambipolar charge transport with electron and hole mobilities of up to 0.34 and 0.38 cm2 V−1 s−1, respectively, which are among the best ambipolar transport characteristics of 1D-MNMs. Furthermore, a complementary inverter based on the ambipolar 1D-MNM of DCP was also constructed with a gain of up to 7, indicating potential application in organic logic circuits. |
Issue Date: | 3-Mar-2023 |
Date of Acceptance: | 14-Dec-2022 |
URI: | http://hdl.handle.net/10044/1/103242 |
DOI: | 10.1007/s40843-022-2364-3 |
ISSN: | 2199-4501 |
Publisher: | Springer |
Start Page: | 2429 |
End Page: | 2435 |
Journal / Book Title: | Science China Materials |
Volume: | 66 |
Copyright Statement: | © Science China Press 2023. This version of the article has been accepted for publication, after peer review (when applicable) and is subject to Springer Nature’s AM terms of use, but is not the Version of Record and does not reflect post-acceptance improvements, or any corrections. The Version of Record is available online at: https://doi.org/10.1007/s40843-022-2364-3 |
Publication Status: | Published |
Online Publication Date: | 2023-03-03 |
Appears in Collections: | Chemistry Faculty of Natural Sciences |