Materials, photophysics and device engineering of perovskite light-emitting diodes
File(s)PeLEDreview_revised manuscript_V1.pdf (25.38 MB)
Accepted version
Author(s)
Chen, Ziming
Li, Zhenchao
Hopper, Thomas
Bakulin, artem
Yip, Hin-Lap
Type
Journal Article
Abstract
Here we provide a comprehensive review of a newly developed lighting technology based on metal halide perovskites (i.e. perovskite light-emitting diodes) encompassing the research endeavours into materials, photophysics and device engineering. At the outset we survey the basic perovskite structures and their various dimensions (namely three-, two- and zero-dimensional perovskites), and demonstrate how the compositional engineering of these structures affects the perovskite light-emitting properties. Next, we turn to the physics underpinning photo- and electroluminescence in these materials through their connection to the fundamental excited states, energy/charge transport processes and radiative and non-radiative decay mechanisms. In the remainder of the review, we focus on the engineering of perovskite light-emitting diodes, including the history of their development as well as an extensive analysis of contemporary strategies for boosting device performance. Key concepts include balancing the electron/hole injection, suppression of parasitic carrier losses, improvement of the photoluminescence quantum yield and enhancement of the light extraction. Overall, this review reflects the current paradigm for perovskite lighting, and is intended to serve as a foundation to materials and device scientists newly working in this field.
Date Issued
2021-04-12
Date Acceptance
2021-03-17
Citation
Reports on Progress in Physics, 2021, 84 (4)
ISSN
0034-4885
Publisher
IOP Publishing
Journal / Book Title
Reports on Progress in Physics
Volume
84
Issue
4
Copyright Statement
© 2021 IOP Publishing Ltd. This is an author-created, un-copyedited version of an article accepted for publication in Reports on Progress in Physics. IOP Publishing Ltd is not responsible for any errors or omissions in this version of the manuscript or any version derived from it. The definitive publisher authenticated version is available online at https://iopscience.iop.org/article/10.1088/1361-6633/abefba
Sponsor
Engineering & Physical Science Research Council (E
Commission of the European Communities
The Royal Society
Grant Number
CHSA_P88115
639750
UF130178
Subjects
Science & Technology
Physical Sciences
Physics, Multidisciplinary
Physics
perovskites
light-emitting diodes
photophysics
device engineering
materials
device engineering
light-emitting diodes
materials
perovskites
photophysics
01 Mathematical Sciences
02 Physical Sciences
General Physics
Publication Status
Published
Article Number
ARTN 046401