In this work, we designed metal-CFRP joints with a profiled adherend termination to improve the mechanical performance. We have applied several profiles to the edge of titanium adherends which were adhesively bonded to CFRP substrates. We conducted finite element modelling and experimental 4PB (4-Point-Bend) testing to investigate how the geometry of the adherend edge profile effects the mechanical performance of the joint. This work shows that profiling of the metal adherend can result in increases of at least 27% in the peak load, and of at least 272% in the energy dissipated up to critical failure normalised by the mechanical energy.