Fluidised bed oxy-fuel gasification of coal: Interactions between volatiles and char at varying pressures and fuel feed rates
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Published version
Author(s)
Long, Xiangyi
Spiegl, Nicolas
Berrueco, Cesar
Paterson, Nigel
Millan, Marcos
Type
Journal Article
Abstract
Fluidised bed gasification is a versatile technology in terms of load flexibility and ability to process various fuels. However, fluidised bed gasification processes are usually air-blown, making integration with CO2 capture difficult and expensive. Operation of a fluidised bed gasifier with O2/recycled CO2 mixtures has been proposed as a route to overcome this drawback. In this work, the effect of pressure and fuel feed rate on the extent of gasification of German lignite in a CO2 rich atmosphere has been examined in a fluidised bed reactor (FBR). A 19% decrease in carbon conversion with increasing pressure from 5 to 20 bara was observed. The higher fuel feeding rates needed to maintain the gasification agent to coal ratio in the FBR at high pressures produces a larger concentration of tars in the reactor, which seems to cause deposition, by intra and inter particle reaction, on the char and reduces its reactivity.
Date Issued
2020-11
Date Acceptance
2020-06-09
Citation
Chemical Engineering Science: X, 2020, 8, pp.1-11
ISSN
2590-1400
Publisher
Elsevier BV
Start Page
1
End Page
11
Journal / Book Title
Chemical Engineering Science: X
Volume
8
Copyright Statement
© 2020 Published by Elsevier Ltd.
This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
Identifier
https://www.sciencedirect.com/science/article/pii/S2590140020300149?via%3Dihub
Publication Status
Published
Article Number
100068
Date Publish Online
2020-06-20