Ferromagnetic resonance and Andreev spectroscopy on exotic superconducting states
File(s)
Author(s)
Chan, Alex Kevin Kar Tsung
Type
Thesis
Abstract
This thesis examines two aspects of superconducting phenomena by employing two different experimental techniques. The first phenomenon is two-gap superconductivity, and the second phenomenon is long-range proximity induced spin-triplet (LRPST) superconductivity.
Using point contact Andreev reflection (PCAR) spectroscopy, evidence for two-gap superconductivity was investigated in Mo1-xRex alloys. Recent specific heat capacity measurements claim the existence of two-gap superconductivity in these alloys. PCAR spectroscopy can identify superconducting energy gaps, and was used here to see if two-gap superconductivity could be confirmed. Direct observation of two distinct energy gaps in spectra measured at 4.2 K and 2 K was not found. However, comparing the temperature dependent PCAR parameters extracted from a single-gap fit with a two-gap fit to the spectra offered some interesting insight.
PCAR spectroscopy was also used to investigate the second phenomenon. In superconductor/ferromagnet (S/F) structures, it is possible to create LRPST with long-range penetration in F by having a spatially inhomogeneous magnetic layer at the interface. This interface is known as a ‘spin-active’ interface, where spin-mixing and spin-rotation processes can occur. Stimulated by claims that a paramagnetic Meissner effect, carried by spin-triplets, can be observed in Nb/Ho/Au multilayers, PCAR was used here to see if signatures of proximity induced spin-triplets could be observed. Theoretical calculations have predicted that spin-mixing at the spin-active interface can lead to Andreev bound states that appear as sub-gap features in electrical conductance spectra. Furthermore, LRPST may also give rise to a peak in the density of states at zero energy.
Finally, a ferromagnetic resonance (FMR) technique was used to see if LRPST could be detected in a non-equilibrium system. Nb/Cr/Fe/Cr/Nb multilayers were studied, where it was found that the key signature of a spin-triplet channel was observed only when the correct conditions were satisfied in the presence of an externally applied field.
Using point contact Andreev reflection (PCAR) spectroscopy, evidence for two-gap superconductivity was investigated in Mo1-xRex alloys. Recent specific heat capacity measurements claim the existence of two-gap superconductivity in these alloys. PCAR spectroscopy can identify superconducting energy gaps, and was used here to see if two-gap superconductivity could be confirmed. Direct observation of two distinct energy gaps in spectra measured at 4.2 K and 2 K was not found. However, comparing the temperature dependent PCAR parameters extracted from a single-gap fit with a two-gap fit to the spectra offered some interesting insight.
PCAR spectroscopy was also used to investigate the second phenomenon. In superconductor/ferromagnet (S/F) structures, it is possible to create LRPST with long-range penetration in F by having a spatially inhomogeneous magnetic layer at the interface. This interface is known as a ‘spin-active’ interface, where spin-mixing and spin-rotation processes can occur. Stimulated by claims that a paramagnetic Meissner effect, carried by spin-triplets, can be observed in Nb/Ho/Au multilayers, PCAR was used here to see if signatures of proximity induced spin-triplets could be observed. Theoretical calculations have predicted that spin-mixing at the spin-active interface can lead to Andreev bound states that appear as sub-gap features in electrical conductance spectra. Furthermore, LRPST may also give rise to a peak in the density of states at zero energy.
Finally, a ferromagnetic resonance (FMR) technique was used to see if LRPST could be detected in a non-equilibrium system. Nb/Cr/Fe/Cr/Nb multilayers were studied, where it was found that the key signature of a spin-triplet channel was observed only when the correct conditions were satisfied in the presence of an externally applied field.
Version
Open Access
Date Issued
2023-05
Date Awarded
2023-09
Copyright Statement
Creative Commons Attribution NonCommercial Licence
License URL
Advisor
Cohen, Lesley
Kurebayashi, Hidekazu
Sponsor
Engineering and Physical Sciences Research Council
Leverhulme Trust
Grant Number
EP/N017242/1
RPG-2016-306
EP/L015277/1
Publisher Department
Materials
Publisher Institution
Imperial College London
Qualification Level
Doctoral
Qualification Name
Doctor of Philosophy (PhD)