Analysis of polarimetric satellite measurements suggests stronger cooling due to aerosol-cloud interactions
File(s)s41467-019-13372-2.pdf (2.51 MB)
Published version
Author(s)
Hasekamp, Otto P
Gryspeerdt, Edward
Quaas, Johannes
Type
Journal Article
Abstract
Anthropogenic aerosol emissions lead to an increase in the amount of Cloud Condensation Nuclei and consequently an increase in cloud droplet number concentration and cloud albedo. The cor-responding negative radiative forcing due to aerosol cloud interactions (RFaci) is one of the most uncertain radiative forcing terms as reported in the 5th Assessment Report of the Intergovernmental Panel on Climate Change (IPCC). We show that previous observation-based studies underestimate aerosol-cloud interactions because they used measurements of aerosol optical properties that are not directly related to cloud formation and are hampered by measurement uncertainties. We have overcome this problem by the use of new polarimetric satellite retrievals of the relevant aerosol properties (aerosol number, size, shape). The resulting estimate of RFaci= -1.14 Wm−2(range be-tween -0.84 and -1.72 Wm−2) is more than a factor 2 stronger than the IPCC estimate that includes
Date Issued
2019-11-27
Date Acceptance
2019-11-04
Citation
Nature Communications, 2019, 9
ISSN
2041-1723
Publisher
Nature Research (part of Springer Nature)
Journal / Book Title
Nature Communications
Volume
9
Copyright Statement
© The Author(s) 2019. This article is licensed under a Creative CommonsAttribution 4.0 International License, which permits use, sharing,adaptation, distribution and reproduction in any medium or format, as long as you giveappropriate credit to the original author(s) and the source, provide a link to the CreativeCommons license, and indicate if changes were made. The images or other third partymaterial in this article are included in the article’s Creative Commons license, unlessindicated otherwise in a credit line to the material. If material is not included in thearticle’s Creative Commons license and your intended use is not permitted by statutoryregulation or exceeds the permitted use, you will need to obtain permission directly fromthe copyright holder. To view a copy of this license, visithttp://creativecommons.org/licenses/by/4.0/.
Publication Status
Published
Article Number
ARTN 5405