Evaluating potential power output of terrestrial thermoradiative diodes with atmospheric modelling
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Published version
Author(s)
Type
Journal Article
Abstract
A thermoradiative diode is a device that can generate power through thermal emission from the warm Earth to the cold night sky. Accurate assessment of the potential power output requires knowledge of the downwelling radiation from the atmosphere. Here, accurate modelling of this radiation is used alongside a detailed balance model of a diode at the Earth’s surface temperature to evaluate its performance under nine different atmospheric conditions. In the radiative limit, these conditions yield power densities between 0.34 and 6.5 W.m-2, with optimal bandgaps near 0.094 eV. Restricting the angles of emission and absorption to less than a full hemisphere can marginally increase the power output. Accounting for non-radiative processes, we suggest that if a 0.094 eV device would have radiative efficiencies more than two orders of magnitude lower than a diode with a bandgap near 0.25 eV, the higher bandgap material is preferred.
Date Issued
2024-12-20
Date Acceptance
2024-11-05
Citation
iScience, 2024, 27 (12)
ISSN
2589-0042
Publisher
Elsevier BV
Journal / Book Title
iScience
Volume
27
Issue
12
Copyright Statement
© 2024 Published by Elsevier Inc. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
Identifier
https://www.sciencedirect.com/science/article/pii/S2589004224025719
Publication Status
Published
Article Number
111346
Date Publish Online
2024-11-09