Interpreting attoclock measurements of tunnelling times
File(s)1402.5620v2.pdf (6.5 MB)
Accepted version
Author(s)
Type
Journal Article
Abstract
Resolving in time the dynamics of light absorption by atoms and molecules, and the electronic rearrangement this induces, is among the most challenging goals of attosecond spectroscopy. The attoclock is an elegant approach to this problem, which encodes ionization times in the strong-field regime. However, the accurate reconstruction of these times from experimental data presents a formidable theoretical task. Here, we solve this problem by combining analytical theory with ab initio numerical simulations. We apply our theory to numerical attoclock experiments on the hydrogen atom to extract ionization time delays and analyse their nature. Strong-field ionization is often viewed as optical tunnelling through the barrier created by the field and the core potential. We show that, in the hydrogen atom, optical tunnelling is instantaneous. We also show how calibrating the attoclock using the hydrogen atom opens the way to identifying possible delays associated with multielectron dynamics during strong-field ionization.
Date Issued
2015-05-25
Date Acceptance
2015-04-21
Citation
Nature Physics, 2015, 11 (6), pp.503-508
ISSN
1745-2481
Publisher
Nature Publishing Group
Start Page
503
End Page
508
Journal / Book Title
Nature Physics
Volume
11
Issue
6
Copyright Statement
Copyright © 2015, Rights Managed by Nature Publishing Group
Sponsor
Engineering & Physical Science Research Council (EPSRC)
Commission of the European Communities
Grant Number
EP/I032517/1
264951
Subjects
Science & Technology
Physical Sciences
Physics, Multidisciplinary
Physics
DELAY-TIME
Publication Status
Published