Barium calcium zirconium titanate thin film-based capacitive thermoelectric converter for low-grade waste heat
File(s)
Published version
Author(s)
Al Thehaiban, Mohammad K
Getov, Vladimir S
Yao, Qiaomu
Ukeje, Chukwudike C
Petrov, Peter K
Type
Journal Article
Abstract
A capacitive thermoelectric device can harvest thermal energy and convert it to electrical energy by employing a
15 temperature-dependent dielectric material whose permittivity sharply changes with temperature. Electricity can be generated by fluctuating the temperature of the capacitor. Currently, capacitive thermoelectric devices are not broadly used, which can be attributed to the low efficiency of the existing solutions, the lack of dielectric materials with suitable temperature non-linearity of the dielectric permittivity, and the complexity of modulating heat flux on the dielectric material. Here, we propose a device based on (Ba0.85Ca0.15)(Ti0.92Zr0.08)O3 and (Ba0.73Ca0.27)(Ti0.98Zr0.02)O3 thin films. The estimated power output under different operation conditions and dynamic workload of an Intel E5-2630 microprocessor show that these thin film materials are promising and can potentially be used for a capacitive thermoelectric converter.
15 temperature-dependent dielectric material whose permittivity sharply changes with temperature. Electricity can be generated by fluctuating the temperature of the capacitor. Currently, capacitive thermoelectric devices are not broadly used, which can be attributed to the low efficiency of the existing solutions, the lack of dielectric materials with suitable temperature non-linearity of the dielectric permittivity, and the complexity of modulating heat flux on the dielectric material. Here, we propose a device based on (Ba0.85Ca0.15)(Ti0.92Zr0.08)O3 and (Ba0.73Ca0.27)(Ti0.98Zr0.02)O3 thin films. The estimated power output under different operation conditions and dynamic workload of an Intel E5-2630 microprocessor show that these thin film materials are promising and can potentially be used for a capacitive thermoelectric converter.
Date Issued
2026-01-07
Date Acceptance
2025-11-14
Citation
Scientific Reports, 2026, 16
ISSN
2045-2322
Publisher
Nature Portfolio
Journal / Book Title
Scientific Reports
Volume
16
Copyright Statement
© The Author(s) 2025 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.
License URL
Publication Status
Published
Article Number
657
Date Publish Online
2026-01-07