High harmonic interferometry of the Lorentz force in strong mid-infrared
laser fields
laser fields
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Published version
Author(s)
Type
Journal Article
Abstract
The interaction of intense mid-infrared laser fields with atoms and molecules
leads to a range of new opportunities, from the production of bright, coherent
radiation in the soft x-ray range to imaging molecular structures and dynamics
with attosecond temporal and sub-angstrom spatial resolution. However, all
these effects, which rely on laser-driven recollision of an electron removed by
the strong laser field and the parent ion, suffer from the rapidly increasing
role of the magnetic field component of the driving pulse: the associated
Lorentz force pushes the electrons off course in their excursion and suppresses
all recollision-based processes, including high harmonic generation, elastic
and inelastic scattering. Here we show how the use of two non-collinear beams
with opposite circular polarizations produces a forwards ellipticity which can
be used to monitor, control, and cancel the effect of the Lorentz force. This
arrangement can thus be used to re-enable recollision-based phenomena in
regimes beyond the long-wavelength breakdown of the dipole approximation, and
it can be used to observe this breakdown in high-harmonic generation using
currently-available light sources.
leads to a range of new opportunities, from the production of bright, coherent
radiation in the soft x-ray range to imaging molecular structures and dynamics
with attosecond temporal and sub-angstrom spatial resolution. However, all
these effects, which rely on laser-driven recollision of an electron removed by
the strong laser field and the parent ion, suffer from the rapidly increasing
role of the magnetic field component of the driving pulse: the associated
Lorentz force pushes the electrons off course in their excursion and suppresses
all recollision-based processes, including high harmonic generation, elastic
and inelastic scattering. Here we show how the use of two non-collinear beams
with opposite circular polarizations produces a forwards ellipticity which can
be used to monitor, control, and cancel the effect of the Lorentz force. This
arrangement can thus be used to re-enable recollision-based phenomena in
regimes beyond the long-wavelength breakdown of the dipole approximation, and
it can be used to observe this breakdown in high-harmonic generation using
currently-available light sources.
Date Issued
2018-05-11
Date Acceptance
2018-04-03
Citation
New Journal of Physics, 2018, 20
ISSN
1367-2630
Publisher
Institute of Physics (IoP) and Deutsche Physikalische Gesellschaft
Journal / Book Title
New Journal of Physics
Volume
20
Copyright Statement
© 2018 The Author(s). Published by IOP Publishing Ltd on behalf of Deutsche Physikalische Gesellschaft. Original content from this work may be used under the terms of the Creative Commons Attribution 3.0 licence. Any further distribution of this work must maintain attribution to the author(s) and the title of the work, journal citation and DOI.
Sponsor
Engineering & Physical Science Research Council (EPSRC)
Identifier
http://arxiv.org/abs/1606.01931v1
Grant Number
EP/N018680/1
Subjects
physics.atom-ph
physics.atom-ph
Publication Status
Published
Article Number
053036