Principles and design of a Zeeman-Sisyphus decelerator for molecular beams
File(s)Fitch_et_al-2016-ChemPhysChem.pdf (4.02 MB)
Published version
Author(s)
Fitch, N
Tarbutt, M
Type
Journal Article
Abstract
We explore a technique for decelerating molecules using a static magnetic eld and optical pumping. Molecules travel through a spatially varying magnetic fi eld and are repeatedly pumped into a weak-field seeking state as they move towards each strong field region, and into a strong-fi eld seeking state as they move towards weak fi eld. The method is time-independent
and so is suitable for decelerating both pulsed and continuous molecular beams. By using guiding magnets at each weak field region, the beam
can be simultaneously guided and decelerated. By tapering the magnetic field strength in the strong field regions, and exploiting the Doppler shift, the velocity distribution can be compressed during deceleration. We develop the principles of this deceleration technique, provide a realistic design, use numerical simulations to evaluate its performance for a beam of CaF, and compare this performance to other deceleration methods.
and so is suitable for decelerating both pulsed and continuous molecular beams. By using guiding magnets at each weak field region, the beam
can be simultaneously guided and decelerated. By tapering the magnetic field strength in the strong field regions, and exploiting the Doppler shift, the velocity distribution can be compressed during deceleration. We develop the principles of this deceleration technique, provide a realistic design, use numerical simulations to evaluate its performance for a beam of CaF, and compare this performance to other deceleration methods.
Date Issued
2016-09-15
Date Acceptance
2016-08-09
Citation
Chemphyschem, 2016, 17 (22), pp.3609-3623
ISSN
1439-7641
Publisher
Wiley-VCH Verlag
Start Page
3609
End Page
3623
Journal / Book Title
Chemphyschem
Volume
17
Issue
22
Copyright Statement
© 2016 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA.This is an open acces s article under the terms of the Creative CommonsAttribution License, which permits use, distribution and reproduction inany medium, provided the original work is properly cited.
Subjects
buffer-gas beams
cold molecules
laser cooling molecules
molecular beam deceleration
optical pumping
physics.atom-ph
Chemical Physics
0306 Physical Chemistry (Incl. Structural)
0202 Atomic, Molecular, Nuclear, Particle And Plasma Physics
0307 Theoretical And Computational Chemistry
Publication Status
Published