Spin-orbit Larmor clock for ionization times in one-photon and strong-field regimes
File(s)1508.00112.pdf (986.53 KB)
Accepted version
Author(s)
Kaushal, J
Morales, F
Torlina, L
Ivanov, M
Smirnova, O
Type
Journal Article
Abstract
Photoionization is a process where absorption of one or several photons liberates an electron and creates a hole in a quantum system, such as an atom or a molecule. Is it faster to remove an electron using one or many photons, and how to define this time? Here we introduce a clock that allows us to define ionization time for both one-photon and many-photon ionization regimes. The clock uses the interaction of the electron or hole spin with the magnetic field created by their orbital motion, known as the spin–orbit interaction. The angle of spin precession in the magnetic field records time. We use the combination of analytical theory and ab initio calculations to show how ionization delay depends on the number of absorbed photons, how it appears in the experiment and what electron dynamics it signifies. In particular, we apply our method to calculate the derived time delays in tunneling regime of strong-field ionization.
Date Issued
2015-12-14
Date Acceptance
2015-08-11
Citation
Journal of Physics B-Atomic Molecular and Optical Physics, 2015, 48 (23)
ISSN
1361-6455
Publisher
IOP Publishing
Journal / Book Title
Journal of Physics B-Atomic Molecular and Optical Physics
Volume
48
Issue
23
Copyright Statement
©2015 IOP Publishing Ltd.
Sponsor
Engineering & Physical Science Research Council (EPSRC)
Commission of the European Communities
Grant Number
EP/I032517/1
264951
Subjects
Science & Technology
Physical Sciences
Optics
Physics, Atomic, Molecular & Chemical
Physics
definition of ionization time
tunneling time
strong-field ionization
attosecond spectroscopy
PHOTOELECTRONS
BARRIER
HELIUM
ATOMS
DELAY
Publication Status
Published
Article Number
234002