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  5. Seeing the unseen: real-time tracking of battery cycling-to-failure via surface strain
 
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Seeing the unseen: real-time tracking of battery cycling-to-failure via surface strain
File(s)
1-s2.0-S2542435125004532-main.pdf (6.05 MB)
Published version (corrected proof)
Author(s)
Gao, Xinlei
Bao, Zemin
Zhang, Lisheng
Brandon, Nigel P
Offer, Gregory J
more
Type
Journal Article
Abstract
Passive failures in lithium-ion batteries, driven by cumulative degradation, present serious safety risks due to their spontaneity and asymptomatic progression. Conventional electrochemical diagnostics cannot differentiate passive failures from routine degradation, while temperature responds too late for early detection. Here, we introduce surface strain as a non-invasive indicator to track degradation-to-failure transitions in commercial 21700 batteries. Under accelerated degradation by depth-of-discharge stress, strain signals detect failure onset > 50% earlier than temperature. We develop two strain-derived metrics, the slope-based threshold and failure-proximity index and achieve 99.7% F1-score (100% true positive rate) and 3.82% normalized mean absolute error for failure detection and proximity estimation using machine learning on partial charging data with strain. Strain monitoring remains effective under fast-charge cycling. Using attachable sensors and lightweight computations, our approach allows easy integration with current battery systems, enabling real-time, onboard passive failure monitoring to enhance battery safety, reliability, and lifespan for future energy storage.
Date Issued
2026-01-02
Date Acceptance
2025-12-03
Citation
Joule, 2026
URI
https://hdl.handle.net/10044/1/126908
URL
https://doi.org/10.1016/j.joule.2025.102272
DOI
10.1016/j.joule.2025.102272
ISSN
2542-4351
Publisher
Elsevier BV
Journal / Book Title
Joule
Copyright Statement
© 2025 The Author(s). Published by Elsevier Inc.
License URL
https://creativecommons.org/licenses/by/4.0/
Publication Status
Published online
Article Number
102272
Date Publish Online
2026-01-02
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