Droplet and percolation network interactions in a fuel cell gas diffusion layer
File(s)Mularczyk et al J Electrochem Soc 2020.pdf (1.31 MB)
Published version
Author(s)
Type
Journal Article
Abstract
Product water accumulations in polymer electrolyte fuel cells can cause performance losses and reactant starvation leading to cell degradation. Liquid water removal in the form of droplets, fed by percolation networks in the gas diffusion layer (GDL), is one of the main transport mechanisms by which the water is evacuated from the GDL. In this study, the effect of droplet detachment in the gas channel on the water cluster inside the GDL has been investigated using X-ray tomographic microscopy and X-ray radiography. The droplet growth is captured in varying stages over a sequence of consecutive droplet releases, during which an inflation and deflation of the gas-liquid interface menisci of the percolating water structure in the GDL has been observed and correlated to changes in pressure fluctuations in the water phase via gas-liquid curvature analysis.
Date Issued
2020-05-01
Date Acceptance
2020-04-01
Citation
Journal of The Electrochemical Society, 2020, 167 (8)
ISSN
0013-4651
Publisher
Electrochemical Society
Journal / Book Title
Journal of The Electrochemical Society
Volume
167
Issue
8
Copyright Statement
© 2020 The Author(s). Published on behalf of The Electrochemical Society by IOP Publishing Limited. This is an open access
article distributed under the terms of the Creative Commons Attribution 4.0 License (CC BY, http://creativecommons.org/licenses/
by/4.0/), which permits unrestricted reuse of the work in any medium, provided the original work is properly cited.
article distributed under the terms of the Creative Commons Attribution 4.0 License (CC BY, http://creativecommons.org/licenses/
by/4.0/), which permits unrestricted reuse of the work in any medium, provided the original work is properly cited.
Identifier
http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000531468600001&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=1ba7043ffcc86c417c072aa74d649202
Subjects
Science & Technology
Physical Sciences
Technology
Electrochemistry
Materials Science, Coatings & Films
Materials Science
LIQUID-WATER
PEMFC
VISUALIZATION
TRANSPORT
FLOW
BREAKTHROUGH
PRESSURE
CHANNELS
SYSTEM
FORCES
Publication Status
Published
Article Number
ARTN 084506
Date Publish Online
2020-04-23