Slowing YbF molecules using radiation pressure
File(s)
Published version
Author(s)
Type
Journal Article
Abstract
We report radiation pressure slowing of YbF molecules to low velocity. In YbF, laser slowing is hindered by leaks out of the optical cycle attributed to low-lying metastable electronic states arising from inner-shell excitation. We bring this population back into the optical cycle once it has decayed to the electronic ground state using microwaves to couple the relevant rotational levels. We measure the scattering rate and closure of the optical cycle as repumps are added, and study the destabilzation of dark states by a magnetic field and by polarization modulation, finding that both are helpful for maximizing the scattering rate. Starting from a beam with a mean speed of 80 m/s, and using frequency broadened slowing light, we reduce the mean speed of the beam and produce a substantial flux in the low velocity tail of the distribution. Slowing increases the fraction of molecules below 40 m/s from 0.4(1)% to 7.0(2)%, and the fraction below 30 m/s from zero to 3.2(1)%. The establishment of a nearly-closed optical cycle and the production of molecules at low velocity are important steps towards trapping YbF molecules for future measurements of the electron’s electric dipole moment.
Date Issued
2025-12-01
Date Acceptance
2025-11-10
Citation
Physical Review Research, 2025, 7 (4)
ISSN
2643-1564
Publisher
American Physical Society
Journal / Book Title
Physical Review Research
Volume
7
Issue
4
Copyright Statement
Published by the American Physical Society Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.
License URL
Publication Status
Published
Article Number
043235
Date Publish Online
2025-12-01