Electrically induced Dirac fermions in graphene nanoribbons
File(s)
Author(s)
Pizzochero, Michele
Tepliakov, Nikita
Mostofi, Arash A
Kaxiras, Efthimios
Type
Journal Article
Abstract
Graphene nanoribbons are widely regarded as promising building blocks for next-generation carbon-based devices. A critical issue to their prospective applications is whether their electronic structure can be externally controlled. Here, we combine simple model Hamiltonians with extensive first-principles calculations to investigate the response of armchair graphene nanoribbons to transverse electric fields. Such fields can be achieved either upon laterally gating the nanoribbon or incorporating ambipolar chemical codopants along the edges. We reveal that the field induces a semiconductor-to-semimetal transition with the semimetallic phase featuring zero-energy Dirac fermions that propagate along the armchair edges. The transition occurs at critical fields that scale inversely with the width of the nanoribbons. These findings are universal to group-IV honeycomb lattices, including silicene and germanene nanoribbons, irrespective of the type of edge termination. Overall, our results create new opportunities to electrically engineer Dirac semimetallic phases in otherwise semiconducting graphene-like nanoribbons.
Date Issued
2021-11-20
Date Acceptance
2021-10-25
Citation
Nano Letters: a journal dedicated to nanoscience and nanotechnology, 2021, 21 (21), pp.9332-9338
ISSN
1530-6984
Publisher
American Chemical Society
Start Page
9332
End Page
9338
Journal / Book Title
Nano Letters: a journal dedicated to nanoscience and nanotechnology
Volume
21
Issue
21
Copyright Statement
Copyright © 2021 American Chemical Society. This document is the Accepted Manuscript version of a Published Work that appeared in final form in Nano Letters, after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acs.nanolett.1c03596
Identifier
https://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000718298700051&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=1ba7043ffcc86c417c072aa74d649202
Subjects
Armchair Graphene Nanoribbons
BAND-GAP
Chemical Doping
Chemistry
Chemistry, Multidisciplinary
Chemistry, Physical
Dirac Fermions
Electric Fields
GROWTH
Materials Science
Materials Science, Multidisciplinary
Nanoelectronics
Nanoscience & Nanotechnology
Physical Sciences
Physics
Physics, Applied
Physics, Condensed Matter
Science & Technology
Science & Technology - Other Topics
Technology
Publication Status
Published
Date Publish Online
2021-10-29