Enhanced quantum sensing with room-temperature solid-state masers.
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Published version
Author(s)
Type
Journal Article
Abstract
Quantum sensing with solid-state electron spin systems finds broad applications in diverse areas ranging from material and biomedical sciences to fundamental physics. Exploiting collective behavior of noninteracting spins holds the promise of pushing the detection limit to even lower levels, while to date, those levels are scarcely reached because of the broadened linewidth and inefficient readout of solid-state spin ensembles. Here, we experimentally demonstrate that such drawbacks can be overcome by a reborn maser technology at room temperature in the solid state. Owing to maser action, we observe a fourfold reduction in the electron paramagnetic resonance linewidth of an inhomogeneously broadened molecular spin ensemble, which is narrower than the same measured from single spins at cryogenic temperatures. The maser-based readout applied to near zero-field magnetometry showcases the measurement signal-to-noise ratio of 133 for single shots. This technique would be an important addition to the toolbox for boosting the sensitivity of solid-state ensemble spin sensors.
Date Issued
2022-12-02
Date Acceptance
2022-10-10
Citation
Science Advances, 2022, 8 (48), pp.1-9
ISSN
2375-2548
Publisher
American Association for the Advancement of Science
Start Page
1
End Page
9
Journal / Book Title
Science Advances
Volume
8
Issue
48
Copyright Statement
Copyright © 2022 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license, which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
Identifier
https://www.ncbi.nlm.nih.gov/pubmed/36449621
Publication Status
Published
Coverage Spatial
United States
Date Publish Online
2022-11-30