How to cool lithium ion batteries: optimising cell design using a thermally coupled model
File(s)J. Electrochem. Soc.-2019-Zhao-A2849-59.pdf (1.53 MB)
Published version
OA Location
Author(s)
Zhao, Yan
Diaz, Laura Bravo
Patel, Yatish
Zhang, Teng
Offer, Gregory J
Type
Journal Article
Abstract
Cooling electrical tabs of the cell instead of the lithium ion cell surfaces has shown to provide better thermal uniformity within the cell, but its ability to remove heat is limited by the heat transfer bottleneck between tab and electrode stack. A two-dimensional electro-thermal model was validated with custom made cells with different tab sizes and position and used to study how heat transfer for tab cooling could be increased. We show for the first time that the heat transfer bottleneck can be opened up with a single modification, increasing the thickness of the tabs, without affecting the electrode stack. A virtual large-capacity automotive cell (based upon the LG Chem E63 cell) was modelled to demonstrate that optimised tab cooling can be as effective in removing heat as surface cooling, while maintaining the benefit of better thermal, current and state-of-charge homogeneity. These findings will enable cell manufacturers to optimise cell design to allow wider introduction of tab cooling. This would enable the benefits of tab cooling, including higher useable capacity, higher power, and a longer lifetime to be possible in a wider range of applications.
Date Issued
2019-08-21
Date Acceptance
2019-08-08
Citation
Journal of The Electrochemical Society, 2019, 166 (13), pp.A2849-A2859
ISSN
0013-4651
Publisher
Electrochemical Society
Start Page
A2849
End Page
A2859
Journal / Book Title
Journal of The Electrochemical Society
Volume
166
Issue
13
Copyright Statement
© The Author(s) 2019. Published by ECS.
http://creativecommons.org/licenses/by/4.0/
This is an open access article distributed under the terms of the Creative Commons Attribution 4.0 License (CC BY, http://creativecommons.org/licenses/by/4.0/), which permits unrestricted reuse of the work in any medium, provided the original work is properly cited.
http://creativecommons.org/licenses/by/4.0/
This is an open access article distributed under the terms of the Creative Commons Attribution 4.0 License (CC BY, http://creativecommons.org/licenses/by/4.0/), which permits unrestricted reuse of the work in any medium, provided the original work is properly cited.
Identifier
http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000482230300003&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=1ba7043ffcc86c417c072aa74d649202
Subjects
Science & Technology
Physical Sciences
Technology
Electrochemistry
Materials Science, Coatings & Films
Materials Science
HEAT-GENERATION
MULTI-PHYSICS
PART II
TEMPERATURE
TAB
DEGRADATION
PERFORMANCE
MANAGEMENT
INHOMOGENEITY
SIMULATION
Publication Status
Published
Date Publish Online
2019-08-21