Non-stationary statistics and formation jitter in transient photon condensation
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Published version
Author(s)
Type
Journal Article
Abstract
While equilibrium phase transitions are easily described by order parameters and free-energy
landscapes, for their non-stationary counterparts these quantities are usually ill-defined. Here,
we probe transient non-equilibrium dynamics of an optically pumped, dye-filled microcavity. We
quench the system to a far-from-equilibrium state and find delayed condensation close to a critical
excitation energy, a transient equivalent of critical slowing down. Besides number fluctuations near
the critical excitation energy, we show that transient phase transitions exhibit timing jitter in the
condensate formation. This jitter is a manifestation of the randomness associated with spontaneous
emission, showing that condensation is a stochastic, rather than deterministic process. Despite the
non-equilibrium character of this phase transition, we construct an effective free-energy landscape
that describes the formation jitter and allows, in principle, its generalization to a wider class of
processes.
landscapes, for their non-stationary counterparts these quantities are usually ill-defined. Here,
we probe transient non-equilibrium dynamics of an optically pumped, dye-filled microcavity. We
quench the system to a far-from-equilibrium state and find delayed condensation close to a critical
excitation energy, a transient equivalent of critical slowing down. Besides number fluctuations near
the critical excitation energy, we show that transient phase transitions exhibit timing jitter in the
condensate formation. This jitter is a manifestation of the randomness associated with spontaneous
emission, showing that condensation is a stochastic, rather than deterministic process. Despite the
non-equilibrium character of this phase transition, we construct an effective free-energy landscape
that describes the formation jitter and allows, in principle, its generalization to a wider class of
processes.
Date Issued
2020-03-13
Date Acceptance
2020-02-17
Citation
Nature Communications, 2020, 11
ISSN
2041-1723
Publisher
Nature Research (part of Springer Nature)
Journal / Book Title
Nature Communications
Volume
11
Copyright Statement
© 2020 The Author(s). This article is licensed under a Creative Commons
Attribution 4.0 International License, which permits use, sharing,
adaptation, distribution and reproduction in any medium or format, as long as you give
appropriate credit to the original author(s) and the source, provide a link to the Creative
Commons license, and indicate if changes were made. The images or other third party
material in this article are included in the article’s Creative Commons license, unless
indicated otherwise in a credit line to the material. If material is not included in the
article’s Creative Commons license and your intended use is not permitted by statutory
regulation or exceeds the permitted use, you will need to obtain permission directly from
the copyright holder. To view a copy of this license, visit http://creativecommons.org/
licenses/by/4.0/.
Attribution 4.0 International License, which permits use, sharing,
adaptation, distribution and reproduction in any medium or format, as long as you give
appropriate credit to the original author(s) and the source, provide a link to the Creative
Commons license, and indicate if changes were made. The images or other third party
material in this article are included in the article’s Creative Commons license, unless
indicated otherwise in a credit line to the material. If material is not included in the
article’s Creative Commons license and your intended use is not permitted by statutory
regulation or exceeds the permitted use, you will need to obtain permission directly from
the copyright holder. To view a copy of this license, visit http://creativecommons.org/
licenses/by/4.0/.
Sponsor
Engineering & Physical Science Research Council (EPSRC)
Commission of the European Communities
Engineering & Physical Science Research Council (EPSRC)
Grant Number
EP/S000755/1
820392
EP/J017027/1
Publication Status
Published
Article Number
1390
Date Publish Online
2020-03-13