This article assesses the state-of-the-art for research on one-part alkali-activated materials, with particular emphasis on recent work dealing with the constituent materials, preparation methods, fresh properties, mechanical properties, and durability characteristics. The review, which covers over 170 studies, first discusses the different precursors, solid activators, admixtures, and aggregates used within such materials. Preparation techniques of one-part alkali-activated materials are then addressed, including pre-mixing treatment, mixing and curing, and 3D-printing. Reaction mechanisms and resulting binding phases are also outlined, followed by a detailed discussion on the fresh, mechanical and durability characteristics. The sensitivity of the compressive strength to different precursors and solid activators with varying chemical compositions, is examined, and predictive strength equations are proposed for common mixes. A brief comparison between the fresh, mechanical and durability characteristics of one-part and two-part AAMs is outlined, followed by a discussion on design standards as well as health and environmental aspects. The review concludes with suggestions for future research for key applications, with due consideration to the projected availability of precursors and the sustainability of solid activators. It is shown that despite the significant recent developments on one-part alkali-activated materials, further progress necessitates future research with a focus on optimising mixes made from precursors other than fly ash and blast furnace slag, as well as detailed investigations on structural members and components.