Investigation of convective transport in the so-called “gas diffusion layer” used in polymer electrolyte fuel cell
File(s)manuscript_r2.pdf (7.47 MB) supp_mat3.pdf (9.97 MB)
Accepted version
Supporting information
Author(s)
Beruski, O
Lopes, T
Kucernak, ARJ
Perez, J
Type
Journal Article
Abstract
Recent experimental data on a fuel-cell-like system revealed insights into the fluid flow in both free and porous media. A computational model is used to investigate the momentum and species transport in such a system, solved using the finite element method. The model consists of a stationary, isothermal, diluted species transport in free and porous media flow. The momentum transport is treated using different formulations, namely, Stokes-Darcy, Darcy-Brinkman, and hybrid Stokes-Brinkman formulations. The species transport is given by the advection equation for a reactant diluted in air. The formulations are compared to each other and to the available experimental data, where it is concluded that the Darcy-Brinkman formulation reproduces the data appropriately. The validated model is used to investigate the contribution of convection in reactant transport in porous media of fuel cells. Convective transport provides a major contribution to reactant distribution in the so-called diffusion media. For a serpentine channel and flow with
Re
=
260
–
590
, convection accounts for 29–58% of total reactant transport to the catalyst layer.
Re
=
260
–
590
, convection accounts for 29–58% of total reactant transport to the catalyst layer.
Date Issued
2017-10-17
Date Acceptance
2017-09-06
Citation
Physical Review Fluids, 2017, 2
ISSN
2469-990X
Publisher
American Physical Society
Journal / Book Title
Physical Review Fluids
Volume
2
Copyright Statement
©2017 American Physical Society
Sponsor
Engineering & Physical Science Research Council (EPSRC)
Engineering & Physical Science Research Council (E
Grant Number
EP/J016454/1
EP/P024807/1
Subjects
Science & Technology
Physical Sciences
Physics, Fluids & Plasmas
Physics
MODELING TRANSPORT
POROUS-MEDIUM
PEMFC GDLS
PERMEABILITY
MEMBRANE
BOUNDARY
FLOW
DISTRIBUTIONS
PERFORMANCE
FLUID
Publication Status
Published
Article Number
103501