Observing spin fractionalization in the Kitaev spin liquid via temperature evolution of indirect resonant inelastic x-ray scattering
File(s)1811.04951v2.pdf (2.98 MB)
Accepted version
Author(s)
Halasz, Gabor B
Kourtis, Stefanos
Knolle, Johannes
Perkins, Natalia B
Type
Journal Article
Abstract
Motivated by the ongoing effort to search for high-resolution signatures of quantum spin liquids, we investigate the temperature dependence of the indirect resonant inelastic x-ray scattering (RIXS) response for the Kitaev honeycomb model. We find that, as a result of spin fractionalization, the RIXS response changes qualitatively at two well-separated temperature scales,
T
L
and
T
H
, which correspond to the characteristic energies of the two kinds of fractionalized excitations,
Z
2
gauge fluxes and Majorana fermions, respectively. While thermally excited
Z
2
gauge fluxes at temperature
T
L
lead to a general broadening and softening of the response, the thermal proliferation of Majorana fermions at temperature
T
H
∼
10
T
L
results in a significant shift of the spectral weight, both in terms of energy and momentum. Due to its exclusively indirect nature, the RIXS process we consider gives rise to a universal magnetic response and, from an experimental perspective, it directly corresponds to the
K
-edge of
Ru
3
+
in the Kitaev candidate material
α
−
RuCl
3
.
T
L
and
T
H
, which correspond to the characteristic energies of the two kinds of fractionalized excitations,
Z
2
gauge fluxes and Majorana fermions, respectively. While thermally excited
Z
2
gauge fluxes at temperature
T
L
lead to a general broadening and softening of the response, the thermal proliferation of Majorana fermions at temperature
T
H
∼
10
T
L
results in a significant shift of the spectral weight, both in terms of energy and momentum. Due to its exclusively indirect nature, the RIXS process we consider gives rise to a universal magnetic response and, from an experimental perspective, it directly corresponds to the
K
-edge of
Ru
3
+
in the Kitaev candidate material
α
−
RuCl
3
.
Date Issued
2019-05-15
Date Acceptance
2019-05-01
Citation
Physical Review B: Condensed Matter and Materials Physics, 2019, 99 (18), pp.184417-1-184417-8
ISSN
1098-0121
Publisher
American Physical Society
Start Page
184417-1
End Page
184417-8
Journal / Book Title
Physical Review B: Condensed Matter and Materials Physics
Volume
99
Issue
18
Copyright Statement
©2019 American Physical Society
Identifier
http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000468206600003&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=1ba7043ffcc86c417c072aa74d649202
Subjects
Science & Technology
Technology
Physical Sciences
Materials Science, Multidisciplinary
Physics, Applied
Physics, Condensed Matter
Materials Science
Physics
LIGHT-SCATTERING
PHYSICS
Publication Status
Published
Article Number
ARTN 184417
Date Publish Online
2019-05-15