Transported probability density function based modelling of soot particle size distributions in non-premixed turbulent jet flames
File(s)Manuscript_PCI_Schiener.pdf (2.86 MB)
Accepted version
Author(s)
Lindstedt, RP
Schiener, MA
Type
Journal Article
Abstract
The need to establish actual particle size distributions (PSDs) of soot emissions from the nanoscale upwards, along with the current global indicators based on soot mass, stems from increasingly strict regulatory demands. In the current work, a mass and number density preserving sectional model is coupled with a transported probability density function (PDF) method to study the evolution of soot PSDs in two non-premixed turbulent jet flames at Reynolds numbers of 10,000 and 20,000. The transported PDF approach is closed at joint-scalar level and includes mass fractions of gas phase species, soot sections, as well as enthalpy, leading to a fully coupled 78-dimensional joint-scalar space, treating interactions between turbulence and gas phase/soot chemistry as well as radiation without further approximation. The gas phase chemistry features 144 reactions, 15 solved and 14 steady-state species and an acetylene-based soot inception model is calibrated using comprehensive detailed chemistry up to pyrene and applied to a well-stirred/plug flow reactor configuration. The derived nucleation rate is subsequently applied in the turbulent flame calculations. Soot surface growth is treated via a PAH analogy and oxidation via O, OH and O2 is accounted for. The sectional model features 62 sections covering particle sizes in the range 0.38 nm ≤ dp ≤ 4.4 µm and includes a model for the collision efficiency of small particles ( ≤ 10 nm) based on the Lennard–Jones potential. The computed results reproduce the evolution of the PSDs with encouraging accuracy. It is also shown that the distribution of soot in mixture fraction space is affected by local extinction events.
Date Issued
2019-01-01
Date Acceptance
2018-06-12
Citation
Proceedings of the Combustion Institute, 2019, 37 (1), pp.1049-1056
ISSN
0082-0784
Publisher
Elsevier
Start Page
1049
End Page
1056
Journal / Book Title
Proceedings of the Combustion Institute
Volume
37
Issue
1
Copyright Statement
© 2018 Elsevier Ltd. All rights reserved. This manuscript is licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International Licence http://creativecommons.org/licenses/by-nc-nd/4.0/
Sponsor
Commission of the European Communities
Identifier
https://www.sciencedirect.com/science/article/pii/S1540748918302712
Grant Number
690724
Subjects
Science & Technology
Physical Sciences
Technology
Thermodynamics
Energy & Fuels
Engineering, Chemical
Engineering, Mechanical
Engineering
Particle size distributions
Turbulent flames
Transported PDF methods
Nucleation rates
Soot surface chemistry
QUADRATURE METHOD
DIFFUSION FLAMES
SURFACE REACTIVITY
AEROSOL DYNAMICS
ETHYLENE FLAMES
LAMINAR
COAGULATION
OXIDATION
PRESSURE
GROWTH
0902 Automotive Engineering
0904 Chemical Engineering
0913 Mechanical Engineering
Publication Status
Published
Date Publish Online
2018-07-04