Enhanced third harmonic generation in single Germanium nanodisks excited at the anapole mode
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Supporting information
Accepted version
Author(s)
Grinblat, G
Li, Y
Nielsen, MP
Oulton, R
Maier, SA
Type
Journal Article
Abstract
We present an all-dielectric germanium nanosystem exhibiting a strong third order
nonlinear response and efficient third harmonic generation in the optical regime. A thin germanium
nanodisk shows a pronounced valley in its scattering cross section close to the dark anapole mode,
while the electric field energy inside the disk is maximized due to high confinement within the
dielectric. We investigate the dependence of the third harmonic signal on disk size and pump
wavelength to reveal the nature of the anapole mode. Each germanium nanodisk generates a high
effective third order susceptibility of
(3) = 4.3 10−9 , corresponding to an associated third
harmonic conversion efficiency of 0.0001% at a wavelength of 1650 nm, which is four orders of
magnitude greater than the case of an unstructured germanium reference film. Furthermore, the
nonlinear conversion via the anapole mode outperforms that via the radiative dipolar resonances
by about one order of magnitude, which is consistent with our numerical simulations. These
findings open new possibilities for the optimization of upconversion processes on the nanoscale
through the appropriate engineering of suitable dielectric materials.
nonlinear response and efficient third harmonic generation in the optical regime. A thin germanium
nanodisk shows a pronounced valley in its scattering cross section close to the dark anapole mode,
while the electric field energy inside the disk is maximized due to high confinement within the
dielectric. We investigate the dependence of the third harmonic signal on disk size and pump
wavelength to reveal the nature of the anapole mode. Each germanium nanodisk generates a high
effective third order susceptibility of
(3) = 4.3 10−9 , corresponding to an associated third
harmonic conversion efficiency of 0.0001% at a wavelength of 1650 nm, which is four orders of
magnitude greater than the case of an unstructured germanium reference film. Furthermore, the
nonlinear conversion via the anapole mode outperforms that via the radiative dipolar resonances
by about one order of magnitude, which is consistent with our numerical simulations. These
findings open new possibilities for the optimization of upconversion processes on the nanoscale
through the appropriate engineering of suitable dielectric materials.
Date Issued
2016-06-24
Date Acceptance
2016-06-22
Citation
Nano Letters, 2016, 16 (7), pp.4635-4640
ISSN
1530-6992
Publisher
American Chemical Society
Start Page
4635
End Page
4640
Journal / Book Title
Nano Letters
Volume
16
Issue
7
Copyright Statement
This document is the Accepted Manuscript version of a Published Work that appeared in final form in Nano Letters, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see http://pubs.acs.org/doi/abs/10.1021/acs.nanolett.6b01958
Sponsor
The Royal Society
Engineering & Physical Science Research Council (EPSRC)
Engineering & Physical Science Research Council (E
Office Of Naval Research (USA)
Grant Number
WM110079
EP/L024926/1
EP/M013812/1
N00014-16-1-2288
Subjects
All-dielectric nanodisks
anapole mode
electric field enhancement
third harmonic generation
Nanoscience & Nanotechnology
MD Multidisciplinary
Publication Status
Published