Dynamical density functional theory with hydrodynamic interactions in confined geometries
File(s)A16.09.0254_Revised_Manuscript.pdf (1.53 MB)
Accepted version
Author(s)
Goddard, BD
Nold, A
Kalliadasis, S
Type
Journal Article
Abstract
We study the dynamics of colloidal fluids in both unconfined geometries and when confined by a hard wall. Under minimal assumptions, we derive a dynamical density functional theory (DDFT) which includes hydrodynamic interactions (HI; bath-mediated forces). By using an efficient numerical scheme based on pseudospectral methods for integro-differential equations, we demonstrate its excellent agreement with the full underlying Langevin equations for systems of hard disks in partial confinement. We further use the derived DDFT formalism to elucidate the crucial effects of HI in confined systems.
Date Issued
2016-12-06
Date Acceptance
2016-11-10
Citation
Journal of Chemical Physics, 2016, 145 (21)
ISSN
1089-7690
Publisher
AIP Publishing
Journal / Book Title
Journal of Chemical Physics
Volume
145
Issue
21
Copyright Statement
© 2016 AIP Publishing
Sponsor
Commission of the European Communities
Engineering & Physical Science Research Council (EPSRC)
Grant Number
247031
EP/L025159/1
Subjects
Chemical Physics
02 Physical Sciences
03 Chemical Sciences
09 Engineering
Publication Status
Published