A lubrication replenishment theory for hydrogels
File(s)d0sm01236j.pdf (4.15 MB)
Published version
OA Location
Author(s)
Porte, Elze
Cann, Philippa
Masen, Marc
Type
Journal Article
Abstract
Hydrogels are suggested as less invasive alternatives to total joint replacements, but their inferior tribological performance compared to articular cartilage remains a barrier to implementation. Existing lubrication theories do not fully characterise the friction response of all hydrogels, and a better insight into the lubrication mechanisms must be established to enable optimised hydrogel performance. We therefore studied the lubricating conditions in a hydrogel contact using fluorescent imaging under simulated physiological sliding conditions. A reciprocating configuration was used to examine the effects of contact dimension and stroke length on the lubricant replenishment in the contact. The results show that the lubrication behaviour is strongly dependent on the contact configurations; When the system operates in a ‘migrating’ configuration, with the stroke length larger than the contact width, the contact is uniformly lubricated and shows low friction; When the contact is in an ‘overlapping’ configuration with a stroke length smaller than the contact width, the contact is not fully replenished, resulting in high friction. The mechanism of non-replenishment at small relative stroke length was also observed in a cartilage contact, indicating that the theory could be generalised to soft porous materials. The lubrication replenishment theory is important for the development of joint replacement materials, as most physiological joints operate under conditions of overlapping contact, meaning steady-state lubrication does not necessarily occur.
Date Issued
2020-10-13
Date Acceptance
2020-09-20
Citation
Soft Matter, 2020, 16 (16), pp.10290-10300
ISSN
1744-683X
Publisher
Royal Society of Chemistry
Start Page
10290
End Page
10300
Journal / Book Title
Soft Matter
Volume
16
Issue
16
Copyright Statement
© The Royal Society of Chemistry 2020. This article is licensed under a Creative Commons Attribution 3.0 Unported Licence (https://creativecommons.org/licenses/by/3.0/)
License URL
Identifier
https://pubs.rsc.org/en/content/articlelanding/2020/SM/D0SM01236J#!divAbstract
Subjects
Chemical Physics
02 Physical Sciences
03 Chemical Sciences
09 Engineering
Publication Status
Published
Date Publish Online
2020-10-13