Effects of beverage carbonation on lubrication mechanisms and mouthfeel
File(s)Carbonation paper_ACCEPTED.pdf (6.84 MB)
Accepted version
Author(s)
Type
Journal Article
Abstract
The perception of carbonation is an important factor in beverage consumption which must be understood in order to develop healthier products. Herein, we study the effects of carbonated water on oral lubrication mechanisms involved in beverage mouthfeel and hence taste perception. Friction was measured in a compliant PDMS-glass contact simulating the tongue-palate interface (under representative speeds and loads), while fluorescence microscopy was used to visualise both the flow of liquid and oral mucosal pellicle coverage.
When carbonated water is entrained into the contact, CO2 cavities form at the inlet, which limit flow and thus reduce the hydrodynamic pressure. Under mixed lubrication conditions, when the fluid film thickness is comparable to the surface roughness, this pressure reduction results in significant increases in friction (>300% greater than under non-carbonated water conditions). Carbonated water is also shown to be more effective than non-carbonated water at debonding the highly lubricious, oral mucosal pellicle, which again results in a significant increase in friction. Both these transient mechanisms of starvation and salivary pellicle removal will modulate the flow of tastants to taste buds and are suggested to be important in the experience of taste and refreshment. For example this may be one reason why flat colas taste sweeter.
When carbonated water is entrained into the contact, CO2 cavities form at the inlet, which limit flow and thus reduce the hydrodynamic pressure. Under mixed lubrication conditions, when the fluid film thickness is comparable to the surface roughness, this pressure reduction results in significant increases in friction (>300% greater than under non-carbonated water conditions). Carbonated water is also shown to be more effective than non-carbonated water at debonding the highly lubricious, oral mucosal pellicle, which again results in a significant increase in friction. Both these transient mechanisms of starvation and salivary pellicle removal will modulate the flow of tastants to taste buds and are suggested to be important in the experience of taste and refreshment. For example this may be one reason why flat colas taste sweeter.
Date Issued
2021-03-15
Date Acceptance
2020-10-20
Citation
Journal of Colloid and Interface Science, 2021, 586 (1), pp.142-151
ISSN
0021-9797
Publisher
Elsevier
Start Page
142
End Page
151
Journal / Book Title
Journal of Colloid and Interface Science
Volume
586
Issue
1
Copyright Statement
© 2020 Elsevier Inc. All rights reserved. This manuscript is licensed under the Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International Licence http://creativecommons.org/licenses/by-nc-nd/4.0/
Identifier
https://www.sciencedirect.com/science/article/pii/S0021979720314193
Subjects
Science & Technology
Physical Sciences
Chemistry, Physical
Chemistry
Carbonation
Beverages
Bubble growth
Salivary lubrication
Fluorescence imaging
Mouthfeel
Friction
Oral Tribology
ELASTOHYDRODYNAMIC LUBRICATION
ORAL SENSATION
TRIBOLOGY
COMPLIANT
WATER
DETACHMENT
SWEETENER
CHAMPAGNE
CONTACTS
RHEOLOGY
Beverages
Bubble growth
Carbonation
Fluorescence imaging
Friction
Mouthfeel
Oral Tribology
Salivary lubrication
Chemical Physics
02 Physical Sciences
03 Chemical Sciences
09 Engineering
Publication Status
Published
Date Publish Online
2020-10-26