Linear ultrafast dynamics of plasmon and magnetic resonances in nanoparticles
File(s)PRBmanuscript_rev.pdf (1.08 MB)
Accepted version
Author(s)
Lazzarini, Carlo Maria
Tadzio, Levato
Fitzgerald, Jamie M
Sanchez-Gil, Jose A
Giannini, Vincenzo
Type
Journal Article
Abstract
In this study we present an analytical description of the ultrafast localized surface plasmon and magnetic resonance dynamics in a single nanoparticle (Ag or Si), driven by an ultrashort (fs time scale) Gaussian pulse. Three possible scenarios have been found depending on the incident field, i.e., pulse duration much shorter than, similar to, and much longer than the localized surface plasmon resonance (LSPR) lifetime. A rich physics arises for
τ
pulse
<
τ
LSPR
, even in the linear regime. The surface plasmon dynamics is manifested as (i) a temporal delay of the surface plasmon excitation with regard to the freely propagating pulse and as (ii) a negative exponential tail after the exciting pulse is over. In addition, for sub-fs pulses clear oscillations in the near-field decay have been observed. A similar scenario has been observed considering a nonabsorbing Si sphere. Nanoparticle resonance dynamics may lead to a wealth of new phenomena and applications in nanophotonics such as multipole order resonance interference, pulse-induced delay or temporal shaping on the fs scale, high harmonic generation, attosecond near-field pulse sources, and electron acceleration from metasurface or 3D engineered nanostructures.
τ
pulse
<
τ
LSPR
, even in the linear regime. The surface plasmon dynamics is manifested as (i) a temporal delay of the surface plasmon excitation with regard to the freely propagating pulse and as (ii) a negative exponential tail after the exciting pulse is over. In addition, for sub-fs pulses clear oscillations in the near-field decay have been observed. A similar scenario has been observed considering a nonabsorbing Si sphere. Nanoparticle resonance dynamics may lead to a wealth of new phenomena and applications in nanophotonics such as multipole order resonance interference, pulse-induced delay or temporal shaping on the fs scale, high harmonic generation, attosecond near-field pulse sources, and electron acceleration from metasurface or 3D engineered nanostructures.
Date Issued
2017-12-05
Date Acceptance
2017-10-22
Citation
Physical review B: Condensed matter and materials physics, 2017, 96 (23)
ISSN
1098-0121
Publisher
American Physical Society
Journal / Book Title
Physical review B: Condensed matter and materials physics
Volume
96
Issue
23
Copyright Statement
©2017 American Physical Society. Linear ultrafast dynamics of plasmon and magnetic resonances in nanoparticles
Carlo Maria Lazzarini, Levato Tadzio, Jamie M. Fitzgerald, José A. Sánchez-Gil, and Vincenzo Giannini
Phys. Rev. B 96, 235407 – Published 5 December 2017
Carlo Maria Lazzarini, Levato Tadzio, Jamie M. Fitzgerald, José A. Sánchez-Gil, and Vincenzo Giannini
Phys. Rev. B 96, 235407 – Published 5 December 2017
Subjects
Science & Technology
Physical Sciences
Physics, Condensed Matter
Physics
FANO RESONANCES
ELECTRON ACCELERATION
FIELD ENHANCEMENT
SURFACE-PLASMONS
POLARITON PULSES
METAL DEFECTS
THIN-FILMS
SILICON
NANOANTENNAS
SCATTERING
Publication Status
Published
Article Number
235407