XUV lasing during strong-field-assisted transient absorption in molecules
File(s)bredtmann_amplification.pdf (1.06 MB)
Accepted version
Author(s)
Bredtmann, T
Chelkowski, S
Bandrauk, AD
Ivanov, M
Type
Journal Article
Abstract
Using ab initio non-Born-Oppenheimer simulations, we demonstrate the amplification of XUV radiation in a high-harmonic-generation-type process using the example of the hydrogen molecular ion. A small fraction of the molecules is pumped to a dissociative excited state from which IR-assisted XUV amplification is observed. We show that starting at sufficiently high IR driving field intensities, the ground-state molecules become quasitransparent for XUV radiation, while due to stabilization, gain from excited states is maintained. While the basic physics should also be observable in atomic media, the main advantage of the investigated molecular laser is, first, efficient lasing from field-free excited states with a high mean angular momentum and, second, the possibility to tune the amplified XUV frequency windows via control of the internuclear distance.
Date Issued
2016-02-04
Date Acceptance
2015-05-18
Citation
Physical Review A, 2016, 93 (2)
ISSN
1094-1622
Publisher
American Physical Society
Journal / Book Title
Physical Review A
Volume
93
Issue
2
Copyright Statement
©2016 American Physical Society. Timm Bredtmann, Szczepan Chelkowski, André D. Bandrauk, and Misha Ivanov
Phys. Rev. A 93, 021402(R) – Published 4 February 2016
Phys. Rev. A 93, 021402(R) – Published 4 February 2016
Sponsor
Engineering & Physical Science Research Council (EPSRC)
Engineering & Physical Science Research Council (EPSRC)
Grant Number
EP/I032517/1
EP/N018680/1
Subjects
Science & Technology
Physical Sciences
Optics
Physics, Atomic, Molecular & Chemical
Physics
SUBFEMTOSECOND PULSE GENERATION
PHASE-MATCHED GENERATION
HIGH-HARMONIC GENERATION
SOFT X-RAYS
WATER-WINDOW
LASER-PULSES
INVERSION
AMPLIFICATION
EMISSION
LIGHT
Publication Status
Published
Article Number
021402