Evidence for a continuous decline in lower stratospheric ozone offsetting ozone layer recovery
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Published version
Author(s)
Type
Journal Article
Abstract
Ozone forms in the Earth's atmosphere from the photodissociation of molecular oxygen, primarily in the tropical stratosphere. It is then transported to the extratropics by the Brewer–Dobson circulation (BDC), forming a protective "ozone layer" around the globe. Human emissions of halogen-containing ozone-depleting substances (hODSs) led to a decline in stratospheric ozone until they were banned by the Montreal Protocol, and since 1998 ozone in the upper stratosphere is rising again, likely the recovery from halogen-induced losses. Total column measurements of ozone between the Earth's surface and the top of the atmosphere indicate that the ozone layer has stopped declining across the globe, but no clear increase has been observed at latitudes between 60° S and 60° N outside the polar regions (60–90°). Here we report evidence from multiple satellite measurements that ozone in the lower stratosphere between 60° S and 60° N has indeed continued to decline since 1998. We find that, even though upper stratospheric ozone is recovering, the continuing downward trend in the lower stratosphere prevails, resulting in a downward trend in stratospheric column ozone between 60° S and 60° N. We find that total column ozone between 60° S and 60° N appears not to have decreased only because of increases in tropospheric column ozone that compensate for the stratospheric decreases. The reasons for the continued reduction of lower stratospheric ozone are not clear; models do not reproduce these trends, and thus the causes now urgently need to be established.
Date Issued
2018-02-06
Date Acceptance
2017-12-18
Citation
Atmospheric Chemistry and Physics, 2018, 18 (2), pp.1379-1394
ISSN
1680-7316
Publisher
Copernicus Publications
Start Page
1379
End Page
1394
Journal / Book Title
Atmospheric Chemistry and Physics
Volume
18
Issue
2
Copyright Statement
© Author(s) 2018. This work is distributed under the Creative Commons Attribution 4.0 License (https://creativecommons.org/licenses/by/4.0/).
Sponsor
Science and Technology Facilities Council
Science and Technology Facilities Council (STFC)
Identifier
http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000424257700001&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=1ba7043ffcc86c417c072aa74d649202
Grant Number
ST-N000838
ST/N000838/1
Subjects
Science & Technology
Physical Sciences
Meteorology & Atmospheric Sciences
MERGED SAGE II
COLUMN OZONE
VERTICAL-DISTRIBUTION
DATA SET
TROPOSPHERIC OZONE
TROPOPAUSE HEIGHT
SOLAR-CYCLE
TRENDS
VARIABILITY
CLIMATE
Publication Status
Published