Magnetic relaxation dynamics driven by the first-order character of magnetocaloric La(Fe,Mn,Si)13.
File(s)Royal Society RelaxFinalForSpiral.docx (3.46 MB)
Accepted version
Author(s)
Type
Journal Article
Abstract
Here, we study the temporal evolution of the magnetic field-driven paramagnetic to ferromagnetic transition in the La(Fe,Mn,Si)13 material family. Three compositions are chosen that show varying strengths of the first-order character of the transition, as determined by the relative magnitude of their magnetic hysteresis and temperature separation between the zero-field transition temperature Tc and the temperature Tcrit, where the transition becomes continuous. Systematic variations in the fixed field, isothermal rate of relaxation are observed as a function of temperature and as a function of the degree of first-order character. The relaxation rate is reduced in more weakly first-order compositions and is also reduced as the temperature is increased towards Tcrit At temperatures above Tcrit, the metastability of the transition vanishes along with its associated temporal dynamics.This article is part of the themed issue 'Taking the temperature of phase transitions in cool materials'.
Date Issued
2016-07-11
Date Acceptance
2016-07-11
Citation
Philosophical Transactions of the Royal Society A: Math Phys Eng Sci, 2016, 374 (2074)
ISSN
1364-503X
Publisher
The Royal Society
Journal / Book Title
Philosophical Transactions of the Royal Society A: Math Phys Eng Sci
Volume
374
Issue
2074
Copyright Statement
© 2016 The Author(s) http://royalsocietypublishing.org/licence
Published by the Royal Society. All rights reserved.
Published by the Royal Society. All rights reserved.
Identifier
PII: rsta.2015.0307
Subjects
magnetic refrigeration
magnetic relaxation
magnetocaloric effect
metamagnetic transition
Publication Status
Published