Higher-order topology in bismuth
Author(s)
Type
Journal Article
Abstract
The mathematical field of topology has become a framework in which to describe the low-energy electronic structure of crystalline solids. Typical of a bulk insulating three-dimensional topological crystal are conducting two-dimensional surface states. This constitutes the topological bulk–boundary correspondence. Here, we establish that the electronic structure of bismuth, an element consistently described as bulk topologically trivial, is in fact topological and follows a generalized bulk–boundary correspondence of higher-order: not the surfaces of the crystal, but its hinges host topologically protected conducting modes. These hinge modes are protected against localization by time-reversal symmetry locally, and globally by the three-fold rotational symmetry and inversion symmetry of the bismuth crystal. We support our claim theoretically and experimentally. Our theoretical analysis is based on symmetry arguments, topological indices, first-principles calculations, and the recently introduced framework of topological quantum chemistry. We provide supporting evidence from two complementary experimental techniques. With scanning-tunnelling spectroscopy, we probe the signatures of the rotational symmetry of the one-dimensional states located at the step edges of the crystal surface. With Josephson interferometry, we demonstrate their universal topological contribution to the electronic transport. Our work establishes bismuth as a higher-order topological insulator.
Date Issued
2018-09
Date Acceptance
2018-06-19
Citation
Nature Physics, 2018, 14 (9), pp.918-924
ISSN
1745-2473
Publisher
Springer Science and Business Media LLC
Start Page
918
End Page
924
Journal / Book Title
Nature Physics
Volume
14
Issue
9
Identifier
http://dx.doi.org/10.1038/s41567-018-0224-7
Subjects
01 Mathematical Sciences
02 Physical Sciences
Fluids & Plasmas
Publication Status
Published
Date Publish Online
2018-07-30