Building and breaking bonds by homogenous nucleation in glass-forming melts leading to transitions in three liquid states
File(s)Materials 2021, 14, 2287 Bonds.pdf (10.25 MB)
Published version
Author(s)
Tournier, Robert F
Ojovan, Michael I
Type
Journal Article
Abstract
The thermal history of melts leads to three liquid states above the melting temperatures Tm containing clusters—bound colloids with two opposite values of enthalpy +Δεlg × ΔHm and −Δεlg × ΔHm and zero. All colloid bonds disconnect at Tn+ > Tm and give rise in congruent materials, through a first-order transition at TLL = Tn+, forming a homogeneous liquid, containing tiny superatoms, built by short-range order. In non-congruent materials, (Tn+) and (TLL) are separated, Tn+ being the temperature of a second order and TLL the temperature of a first-order phase transition. (Tn+) and (TLL) are predicted from the knowledge of solidus and liquidus temperatures using non-classical homogenous nucleation. The first-order transition at TLL gives rise by cooling to a new liquid state containing colloids. Each colloid is a superatom, melted by homogeneous disintegration of nuclei instead of surface melting, and with a Gibbs free energy equal to that of a liquid droplet containing the same magic atom number. Internal and external bond number of colloids increases at Tn+ or from Tn+ to Tg. These liquid enthalpies reveal the natural presence of colloid–colloid bonding and antibonding in glass-forming melts. The Mpemba effect and its inverse exist in all melts and is due to the presence of these three liquid states.
Date Issued
2021-05-01
Date Acceptance
2021-04-26
Citation
Materials, 2021, 14 (9)
ISSN
1996-1944
Publisher
MDPI
Journal / Book Title
Materials
Volume
14
Issue
9
Copyright Statement
© 2021 by the authors.Licensee MDPI, Basel, Switzerland.This article is an open access articledistributed under the terms andconditions of the Creative CommonsAttribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
License URL
Identifier
http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000650567700001&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=1ba7043ffcc86c417c072aa74d649202
Subjects
Science & Technology
Physical Sciences
Technology
Chemistry, Physical
Materials Science, Multidisciplinary
Metallurgy & Metallurgical Engineering
Physics, Applied
Physics, Condensed Matter
Chemistry
Materials Science
Physics
liquid–
liquid transitions
glass phase
amorphous
undercooling
superheating
percolation threshold
microheterogeneity
TWINKLING FRACTAL THEORY
PHASE-TRANSITIONS
TEMPERATURE
WATER
CRYSTALLIZATION
SUPERCLUSTERS
DEPENDENCE
VISCOSITY
Publication Status
Published
Article Number
ARTN 2287