The role of chemo-mechanical modelling in the development of battery technology-a perspective
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Author(s)
Boyce, Adam M
Martinez-Paneda, Emilio
Shearing, Paul R
Type
Journal Article
Abstract
In the race to reduce global CO2 emissions and achieve net-zero, chemomechanics must play a critical role in the technological development of current and next-generation batteries to improve their energy storage capabilities and their lifetime. Many degradation processes arise through mechanics via the development of diffusion-induced stress and volumetric strains within the various constituent materials in a battery. From particle cracking in lithium-ion batteries to lithium dendrite-based fracture of solid electrolytes in solid-state batteries, it is clear that significant barriers exist in the development of these energy storage systems, where chemomechanics plays a central part. To accelerate technological and scientific advances in this area, multi-scale and highly coupled multiphysics modelling must be carried out that includes mechanics-based phenomena. In this perspective article, we provide an introduction to chemomechanical modelling, the various physical problems that it addresses, and the issues that need to be resolved in order to expand its use within the field of battery technology.
Date Issued
2024-07
Date Acceptance
2024-03-21
Citation
JPhys Energy, 2024, 6 (2)
ISSN
2515-7655
Publisher
IOP Publishing
Journal / Book Title
JPhys Energy
Volume
6
Issue
2
Copyright Statement
© 2024 The Author(s). Published by IOP Publishing Ltd. Original content from
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Attribution 4.0 licence.
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this work may be used
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Attribution 4.0 licence.
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License URL
Identifier
https://iopscience.iop.org/article/10.1088/2515-7655/ad3675
Subjects
ANODES
battery
chemomechanical
CRACK-GROWTH
DAMAGE
DEFORMATION
degradation
Energy & Fuels
fracture
FRACTURE
LI-ION BATTERIES
Materials Science
Materials Science, Multidisciplinary
modelling
Science & Technology
Technology
Publication Status
Published
Article Number
021001
Date Publish Online
2024-04-22