Transported JPDF modelling and measurements of soot at elevated pressures
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Published version
Author(s)
Tian, L
Boyette, WR
Lindstedt, RP
Guiberti, TF
Roberts, WL
Type
Journal Article
Abstract
Accurate measurements and modelling of soot formation in turbulent flames at elevated pressures form a crucial step towards design methods that can support the development of practical combustion devices. A mass and number density preserving sectional model is here combined with a transported joint-scalar probability density function (JDPF) method that enables a fully coupled scalar space of soot, gas-phase species and enthalpy. The approach is extended to the KAUST turbulent non-premixed ethylene-nitrogen flames at pressures from 1 to 5 bar via an updated global bimolecular (second order) nucleation step from acetylene to pyrene. The latter accounts for pressure-induced density effects with the rate fitted using comparisons with full detailed chemistry up to 20 bar pressure and with experimental data from a WSR/PFR configuration and laminar premixed flames. Soot surface growth is treated via a PAH analogy and soot oxidation is considered via O, OH and O2 using a Hertz-Knudsen approach. The impact of differential diffusion between soot and gas-phase particles is included by a gradual decline of diffusivity among soot sections. Comparisons with normalised experimental OH-PLIF and PAH-PLIF signals suggest good predictions of the evolution of the flame structure. Good agreement was also found for predicted soot volume statistics at all pressures. The importance of differential diffusion between soot and gas-phase species intensifies with pressure with the impact on PSDs more evident for larger particles which tend to be transported towards the fuel rich centreline leading to reduced soot oxidation.
Date Issued
2023
Date Acceptance
2022-09-13
Citation
Proceedings of the Combustion Institute, 2023, 39 (2), pp.2439-2447
ISSN
0082-0784
Publisher
Elsevier
Start Page
2439
End Page
2447
Journal / Book Title
Proceedings of the Combustion Institute
Volume
39
Issue
2
Copyright Statement
© 2022 The Author(s). Published by Elsevier Inc. on behalf of The Combustion Institute. This is an open
access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/)
access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/)
License URL
Identifier
https://www.webofscience.com/api/gateway?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:001021127700001&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=a2bf6146997ec60c407a63945d4e92bb
Subjects
Differential
diffusion
DIFFUSION FLAMES
Energy & Fuels
Engineering
Engineering, Chemical
Engineering, Mechanical
FIELD
High pressure turbulent flames
OXIDATION
PARTICLE-SIZE DISTRIBUTIONS
Physical Sciences
Science & Technology
Sectional model
Soot nucleation
SURFACE REACTIVITY
Technology
Thermodynamics
Transported PDF methods
TURBULENT
Publication Status
Published
Date Publish Online
2022-10-22