I study several aspects of tests of macrorealism (MR), which for a given data set serves to give a quantitative signal of the presence of a specific notion of non-classical behaviour. The insufficiency of classical understanding underpins both the paradoxes of quantum mechanics, its future technological promise, and so these tests are of interest both foundationally and pragmatically. I derive generalisations of the Leggett-Garg (LG) inequalities and Fine’s theorem, which together establish the necessary and sufficient conditions for macrorealism. First, I extend these conditions to tests involving an arbitrary number of measurement times. Secondly, I generalise them beyond the standard dichotomic variable, to systems described by many-valued variables. I also perform a quantum mechanical analysis examining the interplay of different conditions of MR. I then develop the theoretical framework to support tests of macrorealism in continuous variable systems, where I define variables based on coarse-grainings of position. I calculate temporal correlators for general bound systems, and analyse LG violations within the quantum harmonic oscillator (QHO), in its energy eigenstates and coherent states. I analyse the precise physical mechanisms underpinning the violations in terms of probability currents, Bohm trajectories. Staying within continuous variable systems, we outline a different approach to meeting the invasiveness requirement of LG tests. Reasoning that we may approximately non-invasively measure whether a particle crosses the axis, we measure an object which is related to the standard correlators, and derive a set of macrorealistic inequalities for these modified correlators. We demonstrate violations of these modified LG inequalities for several states within the QHO.