Road traffic is a significant emission source of urban particulate matter (PM). Due to the implementation of exhaust regulatory standards in the UK, PM emissions which arise from the wear of brakes, tyres and the road surface, together with the resuspension of road dust are now predicted to exceed tailpipe emissions. While a growing body of academic literature has developed in recent years, non-exhaust emissions (NEE) remain unregulated and largely understudied, and the impact of powertrain electrification on the vehicle fleet has not been quantified. Thus, the aim of this thesis is to improve our understanding of these important emission sources and to determine the impact of NEE on urban air pollution - both now, and in the future.
A series of highly time-resolved atmospheric measurement campaigns has been undertaken at roadside and background locations to determine roadside traffic increments. These measurements provide a comprehensive dataset of traffic emissions in London, Birmingham and Manchester, incorporating locations with different vehicle mix and speed, during summer and winter periods. PM mass and elemental tracers have been used to estimate the contribution of NEE concentrations using a scaling factor approach. A novel CO2 dilution approach has been undertaken to determine average fleet emission factors (EFs), whilst the impact of electric vehicle regenerative braking has also been simulated.
The results indicate that NEE concentrations and EFs are highly dependent upon meteorological conditions, traffic speed, traffic volume and vehicle class. Brake wear is the dominant source of road traffic PM emissions in congested environments, whilst for each emission source, heavy duty vehicles (HDVs) contribute an order of magnitude greater than light duty vehicles (LDVs). On the other hand, despite the predicted increase in mass, the regenerative braking simulations suggest that passenger vehicles under electric powertrains will reduce brake wear emissions by 65 – 95%. This reduction depends on the assessed drive cycle and vehicle class, highlighting the importance of driving style on future brake wear emissions. The EFs developed in this thesis have been combined with traffic forecasts to project total national emissions in the UK up to 2035 – and can be used to validate the national atmospheric emission inventory.
To conclude, a number of recommendations have been made with respect to air quality measurement strategies and emission policies which are needed to further our understanding of NEE, and to reduce these traffic-related emissions. It is proposed that a multi-disciplinary study should be undertaken encompassing laboratory dynamometer testing, on-vehicle measurements and environmental atmospheric measurements.