Investigation of valence band reconstruction methods for attosecond streaking data from surfaces
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Published version
Author(s)
Drmota, Peter
Marangos, Jon
Greening, Daniel
Tisch, John
Type
Journal Article
Abstract
We analyze simulated streaked valence band photoemission with atomic streaking theory-based reconstruction methods to investigate the differences between atomic gas-phase streaking and valence band surface streaking. The careful distinction between atomic and surface streaking is a prerequisite to justify the application of atomic streaking theory-based reconstruction methods to surface streaking measurements. We show that neglecting the band structure underestimates the width of reconstructed photoelectron wavepackets, consistent with the Fourier transform limit of the band spectrum. We find that a fit of Gaussian wavepackets within the description of atomic streaking is adequate to a limited extent. Systematic errors that depend on the near-infrared skin depth, an inherently surface-specific property, are present in temporal widths of wavepackets reconstructed with atomic streaking theory-based methods.
Date Issued
2019-03-18
Date Acceptance
2019-03-03
Citation
Optics Express, 2019, 27 (7), pp.9394-9402
ISSN
1094-4087
Publisher
Optical Society of America (OSA)
Start Page
9394
End Page
9402
Journal / Book Title
Optics Express
Volume
27
Issue
7
Copyright Statement
© 2019 The Author(s). Published by The Optical Society under the terms of the Creative Commons Attribution 4.0 License. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.
Subjects
0205 Optical Physics
1005 Communications Technologies
0906 Electrical And Electronic Engineering
Optics
Publication Status
Published