Effect of Coulomb impurities on the electronic structure of magic angle twisted bilayer graphene
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Published version
Author(s)
Ramzan, Muhammad Sufyan
Goodwin, Zachary AH
Mostofi, Arash A
Kuc, Agnieszka
Lischner, Johannes
Type
Journal Article
Abstract
In graphene, charged defects break the electron-hole symmetry and can even
give rise to exotic collapse states when the defect charge exceeds a critical
value which is proportional to the Fermi velocity. In this work, we investigate
the electronic properties of twisted bilayer graphene (tBLG) with charged
defects using tight-binding calculations. Like monolayer graphene, tBLG
exhibits linear bands near the Fermi level but with a dramatically reduced
Fermi velocity near the magic angle (approximately 1.1{\deg}). This suggests
that the critical value of the defect charge in magic-angle tBLG should also be
very small. We find that charged defects give rise to significant changes in
the low-energy electronic structure of tBLG. Depending on the defect position
in the moir\'e unit cell, it is possible to open a band gap or to induce an
additional flattening of the low-energy valence and conduction bands. Our
calculations suggest that the collapse states of the two monolayers hybridize
in the twisted bilayer. However, their in-plane localization remains largely
unaffected by the presence of the additional twisted layer because of the
different length scales of the moir\'e lattice and the monolayer collapse state
wavefunctions. These predictions can be tested in scanning tunnelling
spectroscopy experiments.
give rise to exotic collapse states when the defect charge exceeds a critical
value which is proportional to the Fermi velocity. In this work, we investigate
the electronic properties of twisted bilayer graphene (tBLG) with charged
defects using tight-binding calculations. Like monolayer graphene, tBLG
exhibits linear bands near the Fermi level but with a dramatically reduced
Fermi velocity near the magic angle (approximately 1.1{\deg}). This suggests
that the critical value of the defect charge in magic-angle tBLG should also be
very small. We find that charged defects give rise to significant changes in
the low-energy electronic structure of tBLG. Depending on the defect position
in the moir\'e unit cell, it is possible to open a band gap or to induce an
additional flattening of the low-energy valence and conduction bands. Our
calculations suggest that the collapse states of the two monolayers hybridize
in the twisted bilayer. However, their in-plane localization remains largely
unaffected by the presence of the additional twisted layer because of the
different length scales of the moir\'e lattice and the monolayer collapse state
wavefunctions. These predictions can be tested in scanning tunnelling
spectroscopy experiments.
Date Issued
2023-07-10
Date Acceptance
2023-05-23
Citation
npj 2D Materials and Applications, 2023, 7, pp.1-8
ISSN
2397-7132
Publisher
Nature Portfolio
Start Page
1
End Page
8
Journal / Book Title
npj 2D Materials and Applications
Volume
7
Copyright Statement
© The Author(s) 2023. Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
License URL
Identifier
http://arxiv.org/abs/2211.01038v2
Subjects
cond-mat.mes-hall
cond-mat.mtrl-sci
cond-mat.mtrl-sci
Publication Status
Published
Article Number
49
Date Publish Online
2023-07-10