Towards Laser Spectroscopy of Highly Charged Ions: Dynamics of 40Ca+ Ions in a Penning Trap
Author(s)
Bharadia, Shailen
Type
Thesis or dissertation
Abstract
To date, the most successful quantum field theory is quantum electrodynamics
(QED) which offers a fully quantum mechanical description of the electromagnetic
interaction between charged particles. Laboratory tests of the theory
have been performed for a wide range of field strengths and no significant deviation
from the predictions of the theory have been found. For heavy highly
charged ions (HCI), the electric and magnetic fields around the nucleus can
be orders of magnitude higher than those achievable by conventional means
in a laboratory. Therefore, these ions offer a new regime in which the theory
should be tested. For HCI above Z > 60, the ground state hyper fine structure
splitting (HFS) shifts into the optical region, and becomes accessible to laser
light sources. The aim of the SPECTRAP experiment at GSI in Germany,
is to perform laser spectroscopy of the HFS in H-like and Li-like HCI, as a
test of the corresponding bound-state QED calculations. In order for this to
be successful, the weak magnetic HFS transitions need to be measured to a
high precision. This will be accomplished in the SPECTRAP experiment by
trapping and cooling bunches of HCI, such that the relative precision of the
measured transition will be on the level of 10-7, allowing bound-state high order
QED calculations to be tested to the level of a few percent. As fluorescence
rates will be low, a critical final part in preparing the ions in the trap will be
the application of a rotating dipole ('rotating wall') about the magnetic field
axis allowing for compression of the ion cloud in the trap, thereby increasing
the fluorescence collection efficiency and signal to noise for detection.
In London, due to the availability of our own superconducting magnet, we
have performed systematic measurements of the dynamics of laser cooled Ca+
ions confined in a Penning trap driven by a rotating wall. With CCD camera
imaging, we have measured the fluorescence from a cloud of ions, identified
as being a strongly correlated non-neutral plasma, as a function of the rotating
wall drive amplitude, frequency, sense of rotation and trap potential.
We show that a cloud driven at sufficient amplitude reaches a low-slip regime
within the time frame of a single CCD exposure (~ 1s), and that heating resonances
are observed on scanning the rotation frequency. These resonances
are identified as being associated with the axial motion of the ions in the trap
potential, and the lowest order azimuthal plasma modes which are believed
to be excited indirectly by a misalignment of the electric and magnetic fields. By operating the rotating wall in the opposite sense of rotation to that used
for cloud compression, the excitation of these plasma modes is shown to be a
good diagnostic probe of the laser cooled rigid rotation frequency of the cloud,
allowing the number density to be inferred from the measurement. These results
will allow the SPECTRAP collaboration to define a procedure and set of
optimum parameters for use of the rotating wall technique that offers maximum
compression of ions needed for the precision spectroscopy of HCI. These
results have been accepted for publication in Applied Physics B [1], and were
presented at the European Conference for Trapped Ions in September 2010.
The in-vacuum confocal fluorescence collection optical design proved valuable
in alignment of the imaging system outside the magnet, and successful in increasing
the detected fluorescence rates. As a result, the optical design and
techniques employed here, have been successfully transferred to the GSI experiment.
We also present simulations conducted to optimise the transport and in- flight
capture of HCI into the SPECTRAP ion trap from the HITRAP facility at
GSI, and report on the first attempts at trapping singly charged Mg+ and Ar+
ions, testing the ability of the system to capture, localise and cool ions.
(QED) which offers a fully quantum mechanical description of the electromagnetic
interaction between charged particles. Laboratory tests of the theory
have been performed for a wide range of field strengths and no significant deviation
from the predictions of the theory have been found. For heavy highly
charged ions (HCI), the electric and magnetic fields around the nucleus can
be orders of magnitude higher than those achievable by conventional means
in a laboratory. Therefore, these ions offer a new regime in which the theory
should be tested. For HCI above Z > 60, the ground state hyper fine structure
splitting (HFS) shifts into the optical region, and becomes accessible to laser
light sources. The aim of the SPECTRAP experiment at GSI in Germany,
is to perform laser spectroscopy of the HFS in H-like and Li-like HCI, as a
test of the corresponding bound-state QED calculations. In order for this to
be successful, the weak magnetic HFS transitions need to be measured to a
high precision. This will be accomplished in the SPECTRAP experiment by
trapping and cooling bunches of HCI, such that the relative precision of the
measured transition will be on the level of 10-7, allowing bound-state high order
QED calculations to be tested to the level of a few percent. As fluorescence
rates will be low, a critical final part in preparing the ions in the trap will be
the application of a rotating dipole ('rotating wall') about the magnetic field
axis allowing for compression of the ion cloud in the trap, thereby increasing
the fluorescence collection efficiency and signal to noise for detection.
In London, due to the availability of our own superconducting magnet, we
have performed systematic measurements of the dynamics of laser cooled Ca+
ions confined in a Penning trap driven by a rotating wall. With CCD camera
imaging, we have measured the fluorescence from a cloud of ions, identified
as being a strongly correlated non-neutral plasma, as a function of the rotating
wall drive amplitude, frequency, sense of rotation and trap potential.
We show that a cloud driven at sufficient amplitude reaches a low-slip regime
within the time frame of a single CCD exposure (~ 1s), and that heating resonances
are observed on scanning the rotation frequency. These resonances
are identified as being associated with the axial motion of the ions in the trap
potential, and the lowest order azimuthal plasma modes which are believed
to be excited indirectly by a misalignment of the electric and magnetic fields. By operating the rotating wall in the opposite sense of rotation to that used
for cloud compression, the excitation of these plasma modes is shown to be a
good diagnostic probe of the laser cooled rigid rotation frequency of the cloud,
allowing the number density to be inferred from the measurement. These results
will allow the SPECTRAP collaboration to define a procedure and set of
optimum parameters for use of the rotating wall technique that offers maximum
compression of ions needed for the precision spectroscopy of HCI. These
results have been accepted for publication in Applied Physics B [1], and were
presented at the European Conference for Trapped Ions in September 2010.
The in-vacuum confocal fluorescence collection optical design proved valuable
in alignment of the imaging system outside the magnet, and successful in increasing
the detected fluorescence rates. As a result, the optical design and
techniques employed here, have been successfully transferred to the GSI experiment.
We also present simulations conducted to optimise the transport and in- flight
capture of HCI into the SPECTRAP ion trap from the HITRAP facility at
GSI, and report on the first attempts at trapping singly charged Mg+ and Ar+
ions, testing the ability of the system to capture, localise and cool ions.
Date Issued
2011-08
Date Awarded
2011-12
Advisor
Thompson, Richard
Segal, Daniel
Sponsor
Engineering and Physical Sciences Research Council, and the Helmholtz Graduate School for Hadron and Ion Research
Creator
Bharadia, Shailen
Publisher Department
Physics
Publisher Institution
Imperial College London
Qualification Level
Doctoral
Qualification Name
Doctor of Philosophy (PhD)